New Publication in Science Advances
Correlation-driven attosecond photoemission delay in the plasmonic excitation of C60 fullerene
The electron, propagating within the plasmonic potential, accumulates a photoemission delay ranging from 50 to about 300 attoseconds, depending on its kinetic energy. Image: RMT.Bergues
Extreme light confinement in plasmonic nanosystems enables novel applications in photonics, sensor technology, energy harvesting, biology, and quantum information processing. Fullerenes represent an extreme case for nanoplasmonics: They are subnanometer carbon-based molecules showing high-energy and ultrabroad plasmon resonances; however, the fundamental mechanisms driving the plasmonic response and the corresponding collective electron dynamics are still elusive. Here, we uncover the dominant role of electron correlations in the dynamics of the giant plasmon resonance (GPR) of the subnanometer system C60 by using attosecond photoemission chronoscopy. We find a characteristic photoemission delay of up to about 300 attoseconds that is purely induced by coherent large-scale electron correlations in the plasmonic potential. These results provide insights into the nature of the plasmon resonances in subnanometer systems and open perspectives for advancing nanoplasmonic applications.
More information can be found in DESY Press Release, and in the University of Hamburg, CUI: Advance Imaging of Matter Press Release.
The online publication can be found here.